I absolutely adore Breaking Bad. So, why not do this?
Twilight is Walter and Rainbow Dash is Jesse. Maybe Iron Will would be Tuco or something. Discord is on my list for Gus. Organized chaos and all that.
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Pinky as Saul
Oh god Spike with Cerebral Palsy…
Rarity - Marie?
Applejack - Hank?
Spike - Walter Jr?